Removal of Methylene Blue Intensified Ozonation Using a High-Performance Rotating Reactor
Main Article Content
Abstract
The advanced oxidation processes (AOPs) were commonly used in textile dyeing wastewater treatment due to its ability to rapidly degrade dyed compounds. However, its disadvantage is the limited dispersion of ozone in wastewater. To minimize the disadvantage, it is necessary to improve the gas-liquid phase contact to maximize the dispersion of ozone in the wastewater body. Therefore, this study investigated the methylene blue (MB) treatment efficiency in textile dyeing wastewater by performing the ozonation process using a high-performance rotating reactor (HP2R) and compared it with the conventional system. The effect of basic operation parameters such as initial pH, initial methylene blue concentration (Co), rotational speed (ω), and the liquid flow rate (QL) on the decolorization efficiency (η) was evaluated. The results showed that the η of the ozonation using the HP2R reached 98% (pH 8) after only 5 minutes, which was 1.8 times higher than that (54%) of conventional ozonation at the identical period. The decolorization efficiency increased with increasing rotational speed (from 82.0 to 92.5% as ω increased from 30 to 1200 rpm), decreasing liquid flow rate (from 98.0 to 74.9% as QL increased from 0.1 to 0.4 l/min) and decreasing initial concentration of MB (from 98.0 to 88.5% as Co increased from 50 to 200 mg/l). These results show that the combined ozonation in the high-gravity technology can be widely applied to various dyeing wastewater treatment processes in general.
Keywords
Rotating packed bed, ozonation, decolorization, methylene blue, textile dyeing wastewater, HP2R
Article Details
References
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[20] Zequan Zeng, Haikui Zou, Xin Li, Baochang Sun, Jianfeng Chen, and Lei Shao. Ozonation of phenol with O3/Fe(II) in acidic environment in a rotating packed bed. Industrial & Engineering Chemistry Research, 2012, 51, p. 10509 - 10516. https://doi.org/10.1021/ie300476d
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[3] Ribeiro AR, Nunes OC, Pereira MF, Silva AM. An overview on the advanced oxidation process applied for the treatment of water pollutants defined in the recently launched Directive 2013/39/EU. Environ Int, 2015, 75: 33-51. https://doi.org/10.1016/j.envint.2014.10.027
[4] Ramshaw, C. and R.H. Mallinson, Mass transfer process. US Patent No. 4,283,255, 1981.
[5] Cortes Garcia, G.E., J. van der Schaaf, and A.A. Kiss, A review on process intensification in HiGee distillation. Journal of Chemical Technology & Biotechnology, 2017, 92(6): p. 1136-1156. https://doi.org/10.1002/jctb.5206
[6] Burns, J. R., J. N. Jamil, and C. Ramshaw, Process intensification: operating characteristics of rotating packed beds - determination of liquid hold-up for a high-voidage structured packing. Chemical Engineering Science, 2000, 55(13): p. 2401-2415. https://doi.org/10.1016/S0009-2509(99)00520-5
[7] Yuan, M.-H., et al., Removal of ammonia from wastewater by air stripping process in laboratory and pilot scales using a rotating packed bed at ambient temperature. Journal of the Taiwan Institute of Chemical Engineers, 2016, 60: p.488-495. https://doi.org/10.1016/j.jtice.2015.11.016
[8] Krishna Gudena, G. P. Rangaiah, and S. Lakshminarayanan. Optimal design of a rotating packed bed for VOC stripping from contaminated groundwater. Industrial & Engineering Chemistry Research, 2012. 51(2): p.835-847. https://doi.org/10.1021/ie201218w
[9] Sing, S.P., et al., Removal of volatile organic compounds from groundwater using a rotary air stripper. Industrial & Engineering Chemistry Research, 1992. 31(2): p. 574-580. https://doi.org/10.1021/ie00002a019
[10] Yuan, M.-H., et al., Ammonia removal from ammonia-rich wastewater by air stripping using a rotating packed bed. Process Safety and Environmental Protection, 2016. 102: p. 777 - 785. https://doi.org/10.1016/j.psep.2016.06.010
[11] Minh Viet Trinh, Tuan Minh Nguyen, Van Tuyen Trinh, Van Manh Do, Thanh Long Ngo, Yi-Hung Chen, Min-Hao Yuan. Evaluation of the operational factors affecting the stripping efficiency of ammonia from aqueous solution using a high-performance rotating reactor (HP2R). Vietnam Journal of Science and Technology, 2022. 60 (5B): p. 265 - 279.
[12] Nur Athikoh, Eko Yulianto, Andi Wibowo Kinandana, Eva Sasmita, Abdillah Husein Sanjani, Reza Wahyu Mustika, Abiyansyah Putra Pratama, Nur Farida Amalia, Gunawan Gunawan, Muhammad Nur. Reduction of methylene blue by using direct continuous czone. Journal of Environment and Earth Science, 2020, 4, 10, p. 46 - 56.
[13] Chasanah, U., Yulianto, E., Zain, A. Z., Sasmita, E., Restiwijaya, M., Kinandana, A. W., Arianto, F. and Nur, M., Evaluation of titration method on determination of ozone concentration produced by dielectric barrier discharge plasma (DBDP) Technology, Journal of Physics: Conference Series, 2019, 1153. https://doi.org/10.1088/1742-6596/1153/1/012086
[14] Konsowa A. H., Ossman M. E., Chen Y., Crittenden J. C. Decolorization of industrial wastewater by ozonation followed by adsorption on activated carbon. J. Hazard. Mater. 2010; 176, p. 181-185. https://doi.org/10.1016/j.jhazmat.2009.11.010
[15] López-López A., Pic J. S., Benbelkacem H., Debellefontaine H. Influence of t-butanol and of pH on hydrodynamic and mass transfer parameters in an ozonation process. Chem. Eng. Process. 2007; 46, p. 649-655. https://doi.org/10.1016/j.cep.2006.08.010
[16] Shuo Zhanga, Dong Wanga, Shasha Zhanga, Xingwen Zhanga, Pingping Fanb. Ozonation and carbon-assisted ozonation of methylene blue as model compound: Effect of solution pH. Procedia Environmental Science, 2013 (18), p. 493 - 502. https://doi.org/10.1016/j.proenv.2013.04.066
[17] Peng Xu, Tianyang Wu, Yang Xiang, Jimmy Yun, Lei Shao. Enhanced treatment of basic red 46 by ozonation in a rotating packed bed with liquid detention. Process, 2023, 11, 1345. https://doi.org/10.3390/pr11051345
[18] Chia-Chang Lin, Wen - Tzong Liu. Ozone oxidation in a rotating packed bed. Journal of Chemical Technology and Biotechnology, 2003, 78: 138 - 141. https://doi.org/10.1002/jctb.708
[19] Liu, T.; Wang, D.; Liu, H.; Zhao, W.; Wang, W.; Shao, L. Rotating packed bed as a novel disinfection contactor for the inactivation of E. coli by ozone. Chemosphere, 2019, 214, 695-701. https://doi.org/10.1016/j.chemosphere.2018.09.149
[20] Zequan Zeng, Haikui Zou, Xin Li, Baochang Sun, Jianfeng Chen, and Lei Shao. Ozonation of phenol with O3/Fe(II) in acidic environment in a rotating packed bed. Industrial & Engineering Chemistry Research, 2012, 51, p. 10509 - 10516. https://doi.org/10.1021/ie300476d